Publikace ÚTF

A comprehensive study of Interatomic Coulombic Decay in argon dimers: Extracting R-dependent absolute decay rates from the experiment

Rist, J.; Miteva, T.; Gaire, B.; Sann, H.; Trinter, F.; Keiling, M.; Gehrken, N.; Moradmand, A.; Berry, B.; Zohrabi, M.; Kunitski, M.; Ben-Itzhak, I.; Belkacem, A.; Weber, T.; Landers, A. L.; Schöffler, M.; Williams, J. B.; Kolorenč, P.; Gokhberg, K.; Jahnke, T.; Dörner, R.

In this work we present a comprehensive and detailed study of Interatomic Coulombic Decay (ICD) occurring after irradiating argon dimers with XUV-synchrotron radiation. A manifold of different decay channels is observed and the corresponding initial and final states are assigned. Additionally, the effect of nuclear dynamics on the ICD electron spectrum is examined for one specific decay channel. The internuclear distance-dependent width Gamma(R) of the decay is obtained from the measured kinetic energy release distribution of the ions employing a classical nuclear dynamics model.
type:article
journal:Journal of Chemical Physics
volume:482
pages:185-191
year:2017
files:
chemphys.482.185.pdf (1810.16 kB)

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